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Narrow-band coherent anti-stokes Raman signals from broad-band pulses
Journal article   Peer reviewed

Narrow-band coherent anti-stokes Raman signals from broad-band pulses

Dan Oron, Nirit Dudovich, D Yelin and Yaron Silberberg
Physical Review Letters, Vol.88(6)
Feb/2002
url
https://doi.org/10.1103/PhysRevLett.88.063004View
Published (Version of record) Restricted
url
https://ezproxy.weizmann.ac.il/login?url=http://dx.doi.org/10.1103/PhysRevLett.88.063004View
Published (Version of record) Restricted

Abstract

By tailoring the phase of a 100 femtosecond probe pulse we are able to obtain a narrow-band coherent anti-Stokes Raman spectroscopy (CARS) resonant signal with a width of less than 15 cm(-1), which is an order of magnitude narrower than the CARS signal from a transform limited pulse. Thus, by measuring the spectrum of the CARS signal we are able to obtain a high-resolution energy level diagram of the probed sample in spite of the broad femtosecond pulse spectrum.

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